Nuclear reactions charged-particle

Neutron-rich lanthanide isotopes occur in the fission of uranium or plutonium and ate separated during the reprocessing of nuclear fuel wastes (see Nuclearreactors). Lanthanide isotopes can be produced by neutron bombardment, by radioactive decay of neighboring atoms, and by nuclear reactions in accelerators where the rate earths ate bombarded with charged particles. The rare-earth content of solid samples can be determined by neutron... 

All the techniques discussed here involve the atomic nucleus. Three use neutrons, generated either in nuclear reactors or very high energy proton ajccelerators (spallation sources), as the probe beam. They are Neutron Diffraction, Neutron Reflectivity, NR, and Neutron Activation Analysis, NAA. The fourth. Nuclear Reaction Analysis, NRA, uses charged particles from an ion accelerator to produce nuclear reactions. The nature and energy of the resulting products identify the atoms present. Since NRA is performed in RBS apparatus, it could have been included in Chapter 9. We include it here instead because nuclear reactions are involved. 

A beam of charged particles (an ion beam) with an energy from a few hundred keV to several MeV is produced in an accelerator and bombards a sample. Nuclear reactions with low-Z nuclei in the sample are induced by this ion beam. Products of these reactions (typically p, d, t, He, a particles, and y rays) are detected, producing a spectrum of particle yield versus energy. Many (p, a) reactions have energies that are too low for efficient detection. In these cases, the associated y rays are detected instead. Important examples are ... 

Fermi had been fascinated by the discovery of the neutron by James Chadwick in 1932. He gradually switched his research interests to the use of neutrons to produce new types of nuclear reactions, in the hope of discovering new chemical elements or new isotopes of known elements. He had seen at once that the uncharged neutron would not be repelled by the positively-charged atomic nucleus. For that reason the uncharged neutron could penetrate much closer to a nucleus without the need for high-energy particle accelerators. lie discovered that slow neutrons could... 

FIGURE 17.17 When a positively charged particle approaches a nucleus, it is repelled strongly. However, a very fast particle can reach the nucleus before the repulsion turns it aside, and a nuclear reaction may result. 

During the red giant phase of stellar evolution, free neutrons are generated by reactions such as C(a,n) and Ne(a,n) Mg. (The (ot,n) notation signifies a nuclear reaction where an alpha particle combines with the first nucleus and a neutron is ejected to form the second nucleus.) The neutrons, having no charge, can interact with nuclei of any mass at the existing temperatures and can in principle build up the elements to Bi, the heaviest stable element. The steady source of neutrons in the interiors of stable, evolved stars produces what is known as the "s process," the buildup of heavy elements by the slow interaction with a low flux of neutrons. The more rapid "r process" occurs in... 

Neutrons readily induce nuclear reactions, but they always produce nuclides on the high neutron-proton side of the belt of stability. Protons must be added to the nucleus to produce an unstable nuclide with a low neutron-proton ratio. Because protons have positive charges, this means that the bombarding particle must have a positive charge. Nuclear reactions with positively charged particles require projectile particles that possess enough kinetic energy to overcome the electrical repulsion between two positive particles. 

Charge number and mass number are conserved in nuclear reactions, so the missing components can be identified from the atomic numbers of the elements and the charge and mass numbers of elementaiy particles. 

Charged particle activation analysis (CPAA) is based on charged particle induced nuclear reactions producing radionuclides that are identified and quantified by their characteristic decay radiation. CPAA allows trace element determination in the bulk of a solid sample as well characterization of a thin surface layer. 

In contrast to PIXE and RBS, where forces are respectively electromagnetic and electrostatic, this kind of microanalysis uses low range nuclear forces. The analysis is based on the detection of the y-rays emitted from nuclei that are in an excited state following a charged particle induced nuclear reaction. 

In CPAA, the incident charged particle induces nuclear reactions which produce radionuclides, and the characteristic decay radiation of the latter is measured. Qualitative analysis of the radionuclide is achieved by measuring its energy and/or... 

The alpha particle is a helium nucleus produced from the radioactive decay of heavy metals and some nuclear reactions. Alpha decay often occurs among nuclei that have a favorable neutron/proton ratio, but contain too many nucleons for stability. The alpha particle is a massive particle consisting of an assembly of two protons and two neutrons and a resultant charge of +2. 

Neutrons have no electrical charge and have nearly the same mass as a proton (a hydrogen atom nucleus). A neutron is hundreds of times larger than an electron, but one quarter the size of an alpha particle. The source of neutrons is primarily nuclear reactions, such as fission, but they are also produced from the decay of radioactive elements. Because of its size and lack of charge, the neutron is fairly difficult to stop, and has a relatively high penetrating power. 

A—In nuclear reactions the mass of a (3 particle is treated as 0, with a charge of-1. Electrons and (3 particles are the same thing. 

This probability depends on the reacting nnclei and prevailing physical conditions, such as temperature and density. It is easy to understand the relevance of the density the more particles there are per cnbic centimetre, the more frequent are the collisions. The role of the temperatnre is also fundamental. Nuclear reactions require high temperatures, in fact, all the higher as the reacting nuclei carry higher electrical charges, as mentioned above. 

Just to reiterate what we have said, neutron capture is the only valid channel towards the extreme complexity of gold (Z = 79). Reactions involving charged particles are energetically unfavourable and moreover inhibited by insurmountable electrical barriers. Because of the strong electrical repulsion between heavy nuclei (which thus contain many protons), the classic thermonuclear fusion reactions are ineffective, and we are forced to accept the idea that nuclear species beyond iron are produced by a process other than thermonuclear fusion. This process is neutron capture. 

Neon is also used in scintillation counters, neutron fission counters, proportional counters, and ionization chambers for detection of charged particles. Its mixtures with bromine vapors or chlorine are used in Geiger tubes for counting nuclear particles. Helium-neon mixture is used in gas lasers. Some other applications of neon are in antifog devices, electrical current detectors, and lightning arrestors. The gas is also used in welding and preparative reactions. In preparative reactions it provides an inert atmosphere to shield the reaction from air contact. 

Conservation of mass and charge are used when writing nuclear reactions. For example, let s consider what happens when uranium-238 undergoes alpha decay. Uranium-238 has 92 protons and 146 neutrons and is symbolized as After it emits an alpha particle, the nucleus now has a mass number of 234 and an atomic number of 90. 

Irradiation with charged particles accelerated in a cyclotron, while eliminating the problem of long-lived silver isotopes caused by the different nuclear reactions involved, is not feasible for any large-scale study because of the cost involved. Unlike a nuclear reactor, where numerous different samples can be irradiated simultaneously, only a single sample can be irradiated using a cyclotron beam. 

Additional interactions of neutrons with nuclei include die release of charged particles by neutron-induced nuclear disintegration, Commonly known reactions are n-p. n — d. and n—ct. In these cases, the incident neutrons may contribute part of their kinetic energy to the target nucleus to effect the disintegration. Hence, more than mere neutron capture is involved, Then, there is usually a lower threshold for the neutron energy below which the reaction fails to occur, Another important reaction involving neutrons is fission, which may occur under different conditions for eidier slow or fast neutrons with appropriate fissionable material. 

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