Direct Effect of Aerosols on Climate

A controversy with possibly far-reaching consequences concerns the impact of atmospheric particles on the earth s climate. Temperature is one of the most easily monitored indicators of climatic change. Among the many discussions of the effects of aerosols on the global mean temperature, we direct the reader to the monograph by Twomey (1977) and the paper by Toon and Pollack (1980), from which some of the following is taken. 

Liao, H., and J. H. Seinfeld, Effect of Clouds on Direct Aerosol Radiative Forcing of Climate, J. Geophys. Res., 103, 3781-3788... 

The climate effects of atmospheric aerosol particles are a matter of continuous interest in the research community. The aerosol-climate effects are divided into two groups The direct effect represents the ability of the particle population to absorb and scatter short-wave radiation - directly affecting the radiation balance. These direct effects depend primarily on the aerosol optical properties and particle number size distribution, as the particle size significantly affects the scattering efficiency of... 

The main difficulty in understanding the causes of climate change is connected with the impossibility of considering climatic feedbacks sufficiently reliably. Primarily, this refers to cloud-radiation feedback, direct and indirect (by the effect on radiation properties of clouds) impacts of atmospheric aerosols on climate, and the impact of the atmosphere-ocean interaction on climate formation. 

Giorgi F. Bi X. and Qian Y. (2003). Indirect and direct effects of anthropogenic sulfate on the climate of East Asia as simulated with a regional coupled climate-chemistry/aerosol model. Climatic Change, 58, 345-376. 

It is necessary to highlight the effects of aerosols and other chemical species on meteorological parameters, which have many different pathways (direct, semi-direct, and indirect effects, etc.) and they have to be prioritised and considered in on-line coupled modelling systems. Sensitivity studies are needed to understand the relative importance of different feedback mechanisms for different species and conditions relevant to air quality and climate interactions. A concerted action to mobilise and coordinate research in this area is needed. 

Both the number concentrations and sizes of aerosol particles directly affect many of their properties and effects. For example, the ability of particles to serve as nuclei for cloud droplet formation depends on their composition as a function of size, although their effectiveness in any given situation depends also on the number of particles present. Knowledge of these aerosol properties is required to evaluate the indirect effects (Section 4.04.7.3) of aerosol particles on climate, i.e., the effect of aerosol particles on cloud reflectivity and persistence. Therefore much attention has been and continues to be focused on determining particle number concentrations and size distributions. 

Indirect climate effects of aerosols are more complex and more difficult to assess than direct effects because they depend on a chain of phenomena that connect aerosol levels to concentrations of cloud condensation nuclei, cloud condensation nuclei concentrations to cloud droplet number concentrations (and size), and these, in turn, to cloud albedo and cloud lifetime. Changes in the number concentration of aerosols are observed to cause variations in the population and sizes of cloud droplets, which are expected to cause... 

It has become clear only recently that the atmospheric sierosol plays an important role for the climate on earth. It is common to distinguish between direct and indirect effects of the aerosols on the climate. Aerosols effect directly the radiation balance of the earth due to scattering and absorption of electromagnetic radiation (radiative forcing). On the other hand they influence the physics and chemistry of the atmosphere as condensation nuclei for cloud droplets and their chemical reactions with atmospheric trace gases. Though these indirect aerosol effects are difficult to quantify, they are at least as important as the direct radiative forcing. An especially important and complex example for the indirect influence of aerosols on the chemistry and radiation balance of the earth is the role of stratospheric aerosol particles on the polar ozone depletion, which is discussed in more detail below. 

In another study focused on the shielding effects of buildings in a marine environment, the directional impact of marine aerosols was revealed by comparing the level of patina on CLIMAT s copper rod... 

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