Optical heterodyning

M cm at the overlap of the pump and the probe beams, which were focused as shown in Fig. 3. The configuration shown also illustrates the modulation on the pump pulse with a kHz chopper. The transmission signal T(t) is recorded on a fast photomultiplier coupled to a lock-in amplifier (LIA), which is an integral part of the heterodyne optical technique described in detail elsewhere. For a discussion on the role of each element in the dye laser and its specifications, the reader is referred to earlier publications (Kalpouzos et al., 1987 McMorrow et al., 1988a). 

A connnon teclmique used to enliance the signal-to-noise ratio for weak modes is to inject a local oscillator field polarized parallel to the RIKE field at the detector. This local oscillator field is derived from the probe laser and will add coherently to the RIKE field [96]. The relative phase of the local oscillator and the RIKE field is an important parameter in describing the optical heterodyne detected (OHD)-RIKES spectrum. If the local oscillator at the detector is in phase with the probe wave, the heterodyne mtensity is proportional to... 

Tokmakoff A, Lang M J, Larson D S and Fleming G R 1997 Intrinsic optical heterodyne detection of a two-dimensional fifth order Raman response Chem. Phys. Lett. 272 48-54... 

Constantine S, Zhou Y, Morals J and Ziegler L D 1997 Dispersed optical heterodyne birefringence and dichroism of transparent liquids J. Phys. Chem. A 101 5456-62... 

Figure Bl.4.2. (A) Basic components of an astronomical heterodyne receiver. The photomicrograph in (B) presents the heart of a quasi-optical SIS mixer and its associated superconducting timing circuits, while the image in (C) shows the fiilly assembled mixer, as it would be incorporated into a low-temperature cryostat (J Zmuidzinas, private conmumication).

Brown E R, McIntosh K A, Smith F W, Manfra M J and Dennis C L 1993 Measurements of optical-heterodyne conversion in low-temperature grown GaAs Appl. Rhys. Lett. 62 1206-8... 

In optical domain, preamplifier is no more an utopia and is in actual use in fiber communication. However quantum physics prohibits the noiseless cloning of photons an amplifier must have a spectral density of noise greater than 1 photon/spatial mode (a "spatial mode" corresponds to a geometrical extent of A /4). Most likely, an optical heterodyne detector will be limited by the photon noise of the local oscillator and optical preamplifier will not increase the detectivity of the system. 

Since a heterodyne receiver is an amplitude and phase detector, it could nicely be used to correlate optical signals received at various remote sites. The local oscillator can be a single laser distributed by optical fiber to the various sites or local lasers that can be synchronized "a posteriori" by reference to a common source (e.g. a bright star). 

Heterodyne is a very efficient tool for detecting the phase of a "coherent" signal i.e. a signal which has a stable phase relation to the local oscillator. The detector is only limited by the quantum fluctuation of vacuum. This property is common use in coherent lidar. Satellite to satellite optical communications using laser as a local oscillator are under development (Fig. 3). 

The capillary wave frequency is detected by an optical heterodyne technique. The laser beam, quasi-elastically scattered by the capillary wave at the liquid-liquid interface, is accompanied by a Doppler shift. The scattered beam is optically mixed with the diffracted beam from the diffraction grating to generate an optical beat in the mixed light. The beat frequency obtained here is the same as the Doppler shift, i.e., the capillary wave frequency. By selecting the order of the mixed diffracted beam, we can change the wavelength of the observed capillary wave according to Eq. (11). 

In frequency-domain FLIM, the optics and detection system (MCP image intensifier and slow scan CCD camera) are similar to that of time-domain FLIM, except for the light source, which consists of a CW laser and an acousto-optical modulator instead of a pulsed laser. The principle of lifetime measurement is the same as that described in Chapter 6 (Section 6.2.3.1). The phase shift and modulation depth are measured relative to a known fluorescence standard or to scattering of the excitation light. There are two possible modes of detection heterodyne and homodyne detection. 

Diffractive Optics-Based Four-Wave Mixing with Heterodyne Detection... 

FIG U RE 1.10 Schematic representation of the experimental setnp for diffractive optics-hased fonr-wave mixing with heterodyne detection. (From Ogilvie, J. P., Plazanet, M., Dadusc, G., and Miller, R. J. D. 2002. J. Phys. Chem. 109 10460-67. With permission)... 

Dadusc, G., Ogilvie, J. R, Schulenberg, R, Marvet, U., and Miller, R. J. D. 2001. Diffractive optics-based heterodyne-detected four-wave mixing signals of protein motion From protein quakes to ligand escape for myoglobin. Proc. Nat. Acad. Sci. USA 98 6110-6115. 

Levenson, M. D., and Eesley, G. L. 1979. Polarization selective optical heterodyne detection for dramatically improved sensitivity in laser spectroscopy. Appl. Phys. 19 1-17. Librizzi, R, Viapianni, C., Abbruzzetti, S., and Cordone, L. 2002. Residual water modulates the dynamics of the protein and of the external matrix in trehalose-coated MbCO An infrared and flash-photolysis study. J. Chem. Phys. 116 1193-1200. 

Heterodyne detection is widely used to improve the SNR of optical measurements. The additional advantage of heterodyne detection for CARS measurements is that it allows direct extraction of either real or imaginary parts of the susceptibility tensor (Vinergoni et al. 2004 Evans et al. 2004). Being introduced for CARS spectroscopy about 30 years ago (Eesley et al. 1978), heterodyne detection was for a long... 

Eesley, G. L., Levenson, M. D., and Tolies, W. M. 1978. Optically heterodyned coherent Raman spectroscopy. IEEE J. Quant. Electron. 14 45-49. 

Before melting and for some time after only the band at 625 cm of the AA [C4CiIm]+ cation was observed in the 600-630 cm i region. Gradually 603 cm i band due to the GA conformer became stronger. After about 10 min the AA/GA intensity ratio became constant. The interpretation [50] is that the rotational isomers do not interconvert momentarily at the molecular level. Most probably it involves a conversion of a larger local structure as a whole. The existence of such local structures of different rotamers has been found by optical heterodyne-detected Raman-induced Kerr-effect spectroscopy (OHD-RIKES) [82], Coherent anti-Stokes Raman scattering (CARS) [83],... 

Fig. 13.20. Optical heterodyne force microscopy (OHFM) and its application to a copper strip of width 500 nm, thickness 350 nm, on a silicon substrate, with subsequent chemical vapour deposition (CVD) of a silicon oxide layer followed by polishing and evaporation of a chromium layer of uniform thickness 100 nm and flatness better than 10 nm (a) amplitude (b) phase 2.5 [im x 2.5 m. Ultrasonic vibration at fi = 4.190 MHz was applied to the cantilever light of wavelength 830 nm was chopped at fo = 4.193 MHz and focused through the tip to a spot of diameter 2 im with incident mean power 0.5 mW the cantilever resonant frequency was 38 kHz. The non-linear tip-sample interaction generates vibrations of the cantilever at the difference frequency f2 — f = 3 kHz (Tomoda et al. 2003).

Kumano, N., Inagaki, K Kolosov, O. V., and Wright, O. B. (1998). Optical heterodyne force microscopy. IEEE 1998 Ultrasonics Symposium, pp. 1269-72. IEEE, New York. [319]... 

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