Spectroscopy coherent Raman

Eesley G L 1981 Coherent Raman Spectroscopy (Oxford Pergamon)... 

Marowsky G and Smirnov V N (eds) 1992 Coherent Raman Spectroscopy Recent Advances (Berlin Springer)... 

Gomez J S 1996 Coherent Raman spectroscopy Modern Techniques in Raman Spectroscopy ed J J Laserna (New York Wiley) pp 305-42... 

Castellucci E M, Righini R and Foggi P (eds) 1993 Coherent Raman Spectroscopy (Singapore World Scientific)... 

Eesley G L 1978 Coherent Raman spectroscopy J. Quant. Spectrosc. Radiat. Transfer 22 507-76... 

Schaertel S A, Albrecht A C, Lau A and Kummrow A 1994 Interferometric coherent Raman spectroscopy with incoherent light some applications Appi. Rhys. B 59 377-87... 

Schaertel S A and Albrecht A C 1994 Interferometric coherent Raman spectroscopy resonant and non-resonant contributions J. Raman Spectrosc. 25 545-55... 

Chronister E L and Crowell R A 1991 Time-resolved coherent Raman spectroscopy of low-temperature molecular solids in a high-pressure diamond anvil cell Chem. Phys. Lett. 182 27... 

Coherent anti-Stokes Raman spectroscopy (CARS) [59] has also found utility in the detemiination of the internal state distributions of products of chemical reactions. This is one of several coherent Raman spectroscopies based on the... 

Temkin S. I., Suvemev A. A. Evaluation of the CARS spectra of linear molecules in the Keilson-Storer model, In Coherent Raman Spectroscopy. ed. G. Marowsky, V. V. Smirnov, Springer Proceedings in Physics 63, pp. 49-53 (Springer, Berlin) (1992). 

Yamaguchi, S. and Tahara, T. (2005) Interface-specific coherent raman spectroscopy in the frequency domain. 

Eesly, G.L. "Coherent Raman Spectroscopy", Pergammon Press, New York, 1981. 

Eesley, G. L., Levenson, M. D., and Tolies, W. M. 1978. Optically heterodyned coherent Raman spectroscopy. IEEE J. Quant. Electron. 14 45-49. 

Pestov, D., Wang, X., Ariunbold, G. O., Murawski, R. K., Sautenkov, V. A., Dogariu, A., Sokolov, A. V., and Scully, M. O. 2008. Single-shot detection of bacterial endospores via coherent Raman spectroscopy. Proc. Natl. Acad. Sci. USA 105 422-27. 

Several types of time-resolved Raman spectroscopies have been reported and reviewed by Hamaguchi and co-workers and Hamaguchi and Gustafson. These include pump-probe spontaneous and time-resolved coherent Raman spectroscopy of the anti-Stokes and Stokes varieties [coherent anti-Stokes Raman spectroscopy (CARS) and coherent Stokes Raman spectroscopy (CSRS)], respectively). Here we will focus on pump-probe time-resolved spontaneous Raman spectroscopy. 

G.L. Eesley, Coherent Raman spectroscopy (Pergamon Press, Oxford, 1981)... 

By contrast, laser scattering methods now permit temperature composition and flow measurements that are both nonintrusive and give very high spatial resolution. These light scattering methods include laser Raman spectroscopy, laser-induced fluorescence, coherent Raman spectroscopy as well as laser velocimetry... 

Owyoung, A., "High Resolution Coherent Raman Spectroscopy of Gases", 4th International Conference on Laser Spectroscopy, Rottach-Egern, FRG, 11-15 June 1979. 

A number of fifth-order coherent Raman spectroscopies have appeared in recent years (11,43-55), and they can show echo-like behavior (56-60). However, the interpretation of these echoes is more complex than the seventh-order echoes. Moreover, many of these experiments are aimed at low-frequency intermolecular motions only a few look at intramolecular vibrational dephasing (47,48). These experiments are not considered in detail in this chapter but are discussed by Blank et al. (Chapter 10) and Fourkas (Chapter 11). 

II. OVERVIEW OF VIBRATIONAL DEPHASING AND COHERENT RAMAN SPECTROSCOPY... 

An alternate approach is to perform coherent Raman spectroscopy in the time domain rather than in the frequency domain. In this case, a single laser that produces short pulses with sufficient bandwidth to excite all of the Raman modes of interest is employed. One pulse or one pair of time-coincident pulses is used to initiate coherent motion of the intermolecular modes. The time dependence of this coherence is then monitored by another laser pulse, whose timing can be varied to map out the Raman free-induction decay (FID). It should be stressed at this point that the information contained in the Raman FID is identical to that in a low-frequency Raman spectrum and that the two types of data can be interconverted by a straightforward Fourier-transform procedure (12-14). Thus, whether a frequency-domain or a time-domain coherent Raman technique should be employed to study a particular system depends only on practical experimental considerations. 

Hamaguchi, H. and Gustafson, T.L. (1994) Ultrafast time-resolved spontaneous and coherent Raman spectroscopy the structure and dynamics of photogenerated transient species, Arm. Rev. Phys. Chem. 45,... 

Figure 3.6-4 Schematic diagram for a few techniques in nonlinear (coherent) Raman spectroscopy (CSRS Coherent Stokes Raman Spectroscopy SRGS Stimulated Raman Gain Spectroscopy IRS Inverse Raman Spectroscopy (= SRLS Stimulated Raman Loss Spectroscopy) CARS Coherent anti-Stokes Raman Spectroscopy PARS Photoacoustic Raman Spectroscopy).

Applications of non-classical Raman spectroscopy resonance Raman, surface enhanced Raman, and nonlinear coherent Raman spectroscopy ... 

Eesley GL (1981) Coherent Raman Spectroscopy, Pergamon Press, Oxford Efrima S (1985) In Modern Aspects of Electrochemistry, vol 16, Conway BE, White RE, Bockris OM (eds). Plenum, New York, p 253... 

Hopkins, G. A., Maroncelli, M., Nibler, J. W., and Dyke, T. R., Coherent Raman spectroscopy ofHCN complexes, Chem. Phys. Lett. 114, 97-102 (1985). 

Coherent Raman spectroscopy Coherent Raman spectroscopy is a term that refers to a series of closely related nonlinear Raman techniques in which the scattered Raman radiation emerges from the sample as a coherent beam -coherent meaning that the photons are all in phase with one another. The coherent techniques include Stimulated Raman Scattering (SRS), Coherent anti-Stokes Raman Spectroscopy (CARS), Coharent Stokes Raman Spectroscopy (CSRS), and Stimulated Raman Gain Spectroscopy (SRGS). Although most of the nonlinear Raman techniques are also coherent techniques, there is one incoherent nonlinear Raman process called Hyper Raman. 

Rotational reorientation of frans-stilbene in alkane solution at room temperature occurs in the 10 to 30-ps time domain [347]. Rare-gas complexes with trons-stilbene were studied by purely rotational coherence spectroscopy [51,364]. Moreover, the decay kinetics of excited trans-stil-bene-cyclodextrin complexes were examined [366], It is worth mentioning that great progress has also been made in high-resolution spectroscopy [52, 369-372], Resonance coherent Raman spectroscopy showed a large enhancement of the electronic hyperpolarizability of t with respect to ground state trons-stilbene [374]. Vibrational motions were observed with ps transient Raman spectroscopy [375]. 

There are several classes of optical effects induced by an internal perturbation, such as saturation of absorption, coherent Raman spectroscopy, multi-photon absorption processes, coherent transient spectroscopy (see Table 0.3). Section 5.1 of this chapter deals with saturation of absorption and multi-photon absorption processes. Section 5.2 outlines the principles of coherent anti-Stokes Raman spectroscopy (CARS), Raman-induced Kerr effect spectroscopy (RIKES), four-wave mixing (FWM), and photon echo. 

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