Pulsed optically pumped

We measured and analyzed the vertical emission from the resonators under pulsed optical pumping. The experimental setup is illustrated in Fig. 12.8a A Ti/sapphire mode-locked laser was used to optically pump the devices at a center wavelength of 980 nm, repetition rate of 76.6 MHz, and pulse duration of approximately 150 fs. A variable attenuator was used to control the pump power. The average pump power and center wavelength were monitored by a wavemeter, through a 50/50 beamsplitter. The pump beam is focused on the back side of the sample with a 50 x objective lens. A 20 x objective lens is used to collect the vertical emission from the sample and to focus it on an IR camera to obtain the NF intensity pattern and to... 

We have studied, theoretically and experimentally, the characteristics of a novel class of lasers that are based on radial Bragg reflectors. Lasing action with low threshold levels are demonstrated at room temperature under pulsed optical pumping. The observed Q factors are in the order of several thousands. The unique characteristics on these lasers make them promising candidates for numerous applications in telecommunications, sensing, and basic research. 

Davis and co-workers clearly demonstrated that the IF(B -> X) system will lase if a suitable chemical pump source can be found [18,19]. In a pulsed optically pumped laser containing 10 Torr of He they found that IF lased on the (v, J )... 

Figure 10-5. Transient transmission changes AV/Po in PPV for different lime delays between the pump and probe pulse. The pump pulse is a 100 fs laser pulse at 325 nm obtained by frequency doubling ol amplified dye laser pulses, (a) and (b) correspond to different sides of a PPV-film. The spectra in (a) were obtained lor the unoxidized side of the sample while the set of spectra in (b) was measured for the oxidized side of the same sample. The main differences observed are a much lower stimulated emission effect for the oxidized side. The two bottom spectra depict the PL-spectra for comparison. The dashed line indicates the optical absorption (according to Kef. (281).

The levitated laser dye droplet was optically pumped by a pulsed (pulse length 5 ns, repetition rate 10 Hz), frequency-doubled Nd YAG laser (2 = 532 nm) in free-space optical setup. Droplet light emission was collected by a multimode optical fiber placed at an angle of approximately 50° relative to pump laser beam. Collected light was analyzed in a fixed-grating spectrometer with a resolution of FWHM 0.15 nm. 

However, for the dendrimer nanocomposite metallic systems this change in shape was not observed. Again, due to the high stability to intense laser pulses, the anisotropy value of the gold dendrimer nanocomposite, which can be viewed as a measure of the symmetry of the particle, did not change after several repeated cycles of measurements. It is possible that the initial optical pumping of the electron-phonon modes of the metal particles is partially absorbed by the encapsulating PAMAM dendrimer. 

Optical pumping techniques are also very common. The source of the pumping light may be a continuous arclamp, a pulsed flashlamp, another laser, or even focused sunlight. 

The different pumping methods, such as the commonly used current injection or optical pumping electron beam pumping and avalanche breakdown have been studied in detail (for further refs, see and information has been obtained regarding the excitation probabilities of the different interband transitions. The very short laser pulses (less than 10 sec) obtained enable rapid processes and their time dependence to be studied. 

Examples of the optical pumping of solutions of luminescent conjugated polymers include laser action at 596 nm of poly[2-methoxy-5-(2-ethylhexyloxy)-p-phenylenevinylene] (MEH-PPV) using excitation with 6 ns Nd YAG third harmonic pulses (354.7 nm). ° Tuning of hexane solutions of the co-polymer poly(2,2, 5,5 -tetraoctyl-p-terphenyl-4,4 -xylene-vinylene-p-phenylenevinylene) (TOP-PPV) was possible between 414 and 456 mn, similar to the classical coumarin laser dyes. ... 

CARS signal originates from a coherent excitation of vibrational level nsing a pair of optical pulses, tUj ( pump ) and (o ( Stokes ), separated by a freqnency of this vibrational level, Q i.e.. 

We describe beamline ID09B at the European Synchrotron Radiation Facility (ESRF), a laboratory for optical pump and x-ray probe experiments to 100-picosecond resolution. The x-ray source is a narrow-band undulator, which can produce up to 1 x 1010 photons in one pulse. The 3% bandwidth of the undulator is sufficiently monochromatic for most diffraction experiments in liquids. A Ti sapphire femtosecond laser is used for reaction initiation. The laser mns at 896 Hz and the wavelength is tunable between 290-1160 nm. The doubled (400 nm) and tripled wavelength (267 nm) are also available. The x-ray repetition frequency from the synchrotron is reduced to 896 Hz by a chopper. The time delay can be varied from 0 ps to 1 ms, which makes it possible to follow structural processes occurring in a wide range of time scales in one experiment. 

The high intensity of x-ray beams from modern synchrotrons has made it possible to conduct optical pump and x-ray probe experiments to a time resolution of 100 ps, i.e. the limit given by the x-ray pulse length of a synchrotron. In these machines, the brightest... 

In the experiment, the transmission intensities for the excited and the dark sample are determined by the number of x-ray photons (/t) recorded on the detector behind the sample, and we typically accumulate for several pump-probe shots. In the absence of external noise sources the accuracy of such a measurement is governed by the shot noise distribution, which is given by Poisson statistics of the transmitted pulse intensity. Indeed, we have demonstrated that we can suppress the majority of electronic noise in experiment, which validates this rather idealistic treatment [13,14]. Applying the error propagation formula to eq. (1) then delivers the experimental noise of the measurement, and we can thus calculate the signal-to-noise ratio S/N as a function of the input parameters. Most important is hereby the sample concentration nsam at the chosen sample thickness d. Via the occasionally very different absorption cross sections in the optical (pump) and the x-ray (probe) domains it will determine the fraction of excited state species as a function of laser fluence. 

Gas-discharge lamps are used to optically pump the metastable helium atoms into a higher excited electronic state, which has a dipole-allowed transition to the ground state. Only He (2 S) can be pumped selectively, thereby producing pure He(23S) beams. For the heavier rare gases, both metastable states are equally pumped by gas-discharge lamps. The use of cutoff filters to selectively pump one state is not adequate because of the temperature dependence of the filter transmission and the low / numbers of the pumping transition. Metastable neon can be selectively pumped by a continuous wave (cw) dye laser,60 whereas Ar, Kr, and Xe have so far only been selectively pumped by pulsed dye lasers.61... 

The method proposed allows direct absolute measurement of local concentration at the instant of the laser pulse in a low pressure flame. We believe that this method could be applied to higher pressure flames by the use of ultrashort duration laser pulses with the new mode locked dye laser technique. But until the detector technology allows such short time resolutions we think that collisional lifetimes studies must be pursued to obtain more precise evaluation of the fluorescence efficiency, and to have a better understanding of the redistribution phenomena involved in optical pumping. For this purpose we are now studying the decay of resolved fluorescence lines. 

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