Neutron processing

The neutron processes occurring in the core of a fission reactor. Fission of... 

Szilard was the one who made the most serious efforts to enhance research on fission on one hand and to prevent leakage of this information to the outside on the other hand. It became apparent by April 1939 that there are two distinct processes which invite further research. The slow neutron process (i.e., a chain reaction in which the fission is induced by slow neutrons) which is suited, probably, only for power production, and the fast neutron process which may cause heavy and violent explosions. 

Name four neutron processes that affect the value of the multiplication factor in the Hanford (or any) reactor. 

It is to use a PC for the random neutron process measurement covering up to four neutron counters. There are various methods of the random neutron process measurement such as correlation, variance to mean ratio, count probability, dead time methods, etc. Each method measures neutron pulse sequence information and obtains reactor dynamic parameters, but the instrumentation or analysis method of each case is different. 

The complex neutron processes can be described by characteristic lengths. They are a measure of the rectified distance travelled by a neutron in its zigzag path between the start and end of consideration. A detailed descriptimi is given, for example, by Ellis et al. (2003), Ellis and Singer (2007) and Gilchrist (2009) ... 

Numerous nuclear transformations have been induced by processes in which atoms have been bombarded with neutrons, protons, deuterium, carbon atoms and ions. 

Fm and heavier isotopes can be produced by intense neutron irradiation of lower elements, such as plutonium, using a process of successive neutron capture interspersed with beta decays until these mass numbers and atomic numbers are reached. 

When hydrogen is burned up in the nuclear furnace of a star, helium burning takes over, forming carbon, which in turn leads to oxygen, etc. Subsequent emission processes releasing a-particles, equilibrium processes, neutron absorption, proton capture, etc. lead to heavier elements. 

Neutron Activation Analysis Few samples of interest are naturally radioactive. For many elements, however, radioactivity may be induced by irradiating the sample with neutrons in a process called neutron activation analysis (NAA). The radioactive element formed by neutron activation decays to a stable isotope by emitting gamma rays and, if necessary, other nuclear particles. The rate of gamma-ray emission is proportional to the analyte s initial concentration in the sample. For example, when a sample containing nonradioactive 13AI is placed in a nuclear reactor and irradiated with neutrons, the following nuclear reaction results. 

It is possible to prepare very heavy elements in thermonuclear explosions, owing to the very intense, although brief (order of a microsecond), neutron flux furnished by the explosion (3,13). Einsteinium and fermium were first produced in this way they were discovered in the fallout materials from the first thermonuclear explosion (the "Mike" shot) staged in the Pacific in November 1952. It is possible that elements having atomic numbers greater than 100 would have been found had the debris been examined very soon after the explosion. The preparative process involved is multiple neutron capture in the uranium in the device, which is followed by a sequence of beta decays. Eor example, the synthesis of EM in the Mike explosion was via the production of from followed by a long chain of short-Hved beta decays,... 

In the spring of 1989, it was announced that electrochemists at the University of Utah had produced a sustained nuclear fusion reaction at room temperature, using simple equipment available in any high school laboratory. The process, referred to as cold fusion, consists of loading deuterium into pieces of palladium metal by electrolysis of heavy water, E)20, thereby developing a sufficiently large density of deuterium nuclei in the metal lattice to cause fusion between these nuclei to occur. These results have proven extremely difficult to confirm (20,21). Neutrons usually have not been detected in cold fusion experiments, so that the D-D fusion reaction familiar to nuclear physicists does not seem to be the explanation for the experimental results, which typically involve the release of heat and sometimes gamma rays. 

A development in the 1960s was that of on-line elemental analysis of slurries using x-ray fluorescence. These have become the industry standard. Both in-stream probes and centralized analyzers are available. The latter is used in large-scale operations. The success of the analyzer depends on how representative the sample is and how accurate the caUbration standards are. Neutron activation analyzers are also available (45,51). These are especially suitable for light element analysis. On-stream analyzers are used extensively in base metal flotation plants as well as in coal plants for ash analysis. Although elemental analysis provides important data, it does not provide information on mineral composition which is most cmcial for all separation processes. Devices that can give mineral composition are under development. 

Nuclear wastes are classified according to the level of radioactivity. Low level wastes (LLW) from reactors arise primarily from the cooling water, either because of leakage from fuel or activation of impurities by neutron absorption. Most LLW will be disposed of in near-surface faciHties at various locations around the United States. Mixed wastes are those having both a ha2ardous and a radioactive component. Transuranic (TRU) waste containing plutonium comes from chemical processes related to nuclear weapons production. These are to be placed in underground salt deposits in New Mexico (see... 

The nuclear chain reaction can be modeled mathematically by considering the probable fates of a typical fast neutron released in the system. This neutron may make one or more coUisions, which result in scattering or absorption, either in fuel or nonfuel materials. If the neutron is absorbed in fuel and fission occurs, new neutrons are produced. A neutron may also escape from the core in free flight, a process called leakage. The state of the reactor can be defined by the multiplication factor, k, the net number of neutrons produced in one cycle. If k is exactly 1, the reactor is said to be critical if / < 1, it is subcritical if / > 1, it is supercritical. The neutron population and the reactor power depend on the difference between k and 1, ie, bk = k — K closely related quantity is the reactivity, p = bk jk. i the reactivity is negative, the number of neutrons declines with time if p = 0, the number remains constant if p is positive, there is a growth in population. 

The analysis of steady-state and transient reactor behavior requires the calculation of reaction rates of neutrons with various materials. If the number density of neutrons at a point is n and their characteristic speed is v, a flux effective area of a nucleus as a cross section O, and a target atom number density N, a macroscopic cross section E = Na can be defined, and the reaction rate per unit volume is R = 0S. This relation may be appHed to the processes of neutron scattering, absorption, and fission in balance equations lea ding to predictions of or to the determination of flux distribution. The consumption of nuclear fuels is governed by time-dependent differential equations analogous to those of Bateman for radioactive decay chains. The rate of change in number of atoms N owing to absorption is as follows ... 

The Natural Reactor. Some two biUion years ago, uranium had a much higher (ca 3%) fraction of U than that of modem times (0.7%). There is a difference in half-hves of the two principal uranium isotopes, U having a half-life of 7.08 x 10 yr and U 4.43 x 10 yr. A natural reactor existed, long before the dinosaurs were extinct and before humans appeared on the earth, in the African state of Gabon, near Oklo. Conditions were favorable for a neutron chain reaction involving only uranium and water. Evidence that this process continued intermittently over thousands of years is provided by concentration measurements of fission products and plutonium isotopes. Usehil information about retention or migration of radioactive wastes can be gleaned from studies of this natural reactor and its products (12). 

Radioactivity occurs naturally in earth minerals containing uranium and thorium. It also results from two principal processes arising from bombardment of atomic nuclei by particles such as neutrons, ie, activation and fission. Activation involves the absorption of a neutron by a stable nucleus to form an unstable nucleus. An example is the neutron reaction of a neutron and cobalt-59 to yield cobalt-60 [10198 0-0] Co, a 5.26-yr half-life gamma-ray emitter. Another is the absorption of a neutron by uranium-238 [24678-82-8] to produce plutonium-239 [15117 8-5], Pu, as occurs in the fuel of a nuclear... 

---