Fission fragment

Desorption ionization (DI). General term to encompass the various procedures (e.g., secondary ion mass spectrometry, fast-atom bombardment, californium fission fragment desorption, thermal desorption) in which ions are generated directly from a solid or liquid sample by energy input. Experimental conditions must be clearly stated. 

The nuclear reactor is a device in which a controlled chain reaction takes place involving neutrons and a heavy element such as uranium. Neutrons are typically absorbed in uranium-235 [15117-96-17, or plutonium-239 [15117 8-5], Pu, nuclei. These nuclei spHt, releasing two fission fragment nuclei... 

Many of the uranium fission fragments are radioactive. Of special interest are technetium-99 [14133-76-7] and iodine-129 [15046-84-1] having half-Hves of 2.13 X 10 yr and 1.7 x 10 yr, respectively. Data on all isotopes are found in Reference 6 (see also Radioisotopes). 

A large number of radiometric techniques have been developed for Pu analysis on tracer, biochemical, and environmental samples (119,120). In general the a-particles of most Pu isotopes are detected by gas-proportional, surface-barrier, or scintillation detectors. When the level of Pu is lower than 10 g/g sample, radiometric techniques must be enhanced by preliminary extraction of the Pu to concentrate the Pu and separate it from other radioisotopes (121,122). Alternatively, fission—fragment track detection can detect Pu at a level of 10 g/g sample or better (123). Chemical concentration of Pu from urine, neutron irradiation in a research reactor, followed by fission track detection, can achieve a sensitivity for Pu of better than 1 mBq/L (4 X 10 g/g sample) (124). 

Track-etched membranes are made by exposing thin films (mica, polycarbonate, etc) to fission fragments from a radiation source. The high energy particles chemically alter material in their path. The material is then dissolved by suitable reagents, leaving nearly cylindrical holes (19). 

Kinetic energy of fission fragments Instantaneous y-rays Kinetic energy of fission neutrons Radioactive decay of fission fragments, P energy Radioactive decay of fission fragments, y energy... 

Nuclear reactors, however, do generate highly radioactive waste. This waste, which consists primarily of the fission fragments and their radioactive-decay products, must be stored for many years before its radioactivity decays to a reasonable level, and the safe long-term storage of this waste is a matter of great concern and debate. Fortunately, the volume of waste that is created is only about 20 cubic meters annually from a reactor, compared with 200,000 cubic meters of waste ash from a coal-fired plant. When nuclear weapions were tested in the atmosphere, the radioactive products from the nuclear explosions were released into the air and fell to Earth as radioactive fallout. 

Alpha particles, multiple-charged particles, fission fragments and heavy particles of unknown charge 20 0.05... 

X-rays, often used in radiation chemistry, differ from y-rays only operationally namely, X-rays are produced in machines, whereas y-rays originate in nuclear transitions. In their interaction with matter, they behave similarly—that is, as a photon of appropriate energy. Other radiations used in radiation-chemical studies include protons, deuterons, various accelerated stripped nuclei, fission fragments, and radioactive radiations (a, /, or y). 

LET of a fission fragment starts at a very high value but is quickly reduced because of electron capture, resulting in an average of-200-300 eV/A. 

FIGURE 3.10 A typical fission fragment track in water, showing dense overlap of secondary electrons in the penumbra region (shaded). Core is shown dotted. Reproduced from Mozumder (1969), by permission of John Wiley Sons, Inc. ... 

Fission chambers use neutron-induced fission to detect neutrons. The chamber is usually similar in construction to that of an ionization chamber, except that the coating material is highly enriched U235. The neutrons interact with the U235, causing fission. One of the two fission fragments enters the chamber, while the other fission fragment embeds itself in the chamber wall. 

A highly positive charged fission fragment interacts with the detector gas and causes ionizations. 

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