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Initial-state nuclear characteristics

Initial-State Nuclear Characteristics of Two-Region, Homogeneous, Molten Fluoride-Salt Reactors Fueled with... [Pg.630]

Initial-State Nuclear Characteristics of Two-Region, Homogeneous, Molten Fluoride-Salt Reactors Fueled with Fuel salt No. 2 37 mole % BeF2 + 63 mole % LiF -h UF4 + TI1F4. [Pg.638]

Here E, and T" are the energy, total width and neutron width of the ith compound resonance, respectively v is the nuclear weak matrix element. The presence of the penetration factor (E E y -kR in eq. (3.4) is characteristic of all correlations observed in low energy nuclear reactions which arise due to initial state interference and, consequently, are proportional to the neutron momentum (the correlation o- iHn the case considered). [Pg.83]

From a theoretical perspective, the object that is initially created in the excited state is a coherent superposition of all the wavefunctions encompassed by the broad frequency spread of the laser. Because the laser pulse is so short in comparison with the characteristic nuclear dynamical time scales of the motion, each excited wavefunction is prepared with a definite phase relation with respect to all the others in the superposition. It is this initial coherence and its rate of dissipation which determine all spectroscopic and collisional properties of the molecule as it evolves over a femtosecond time scale. For IBr, the nascent superposition state, or wavepacket, spreads and executes either periodic vibrational motion as it oscillates between the inner and outer turning points of the bound potential, or dissociates to form separated atoms, as indicated by the trajectories shown in Figure 1.3. [Pg.9]

Initially an extensive literature search was conducted to identify key world oil shales, i.e., deposits of large size and/or of current interest to potential developers. The resulting information was used to select a few key world oil shales. Thirteen oil shale samples from eight different countries were studied. Samples were acquired from each of the following countries Australia, Brazil, Israel, Sweden, the United States, and Yugoslavia. Two samples were acquired from Morocco and five samples were acquired fr qj the People s Republic of China. Fischer, Ultimate, Rock-Eval, C Nuclear Magnetic Resonance Spectroscopy (NMR), and X-ray Diffraction Mineral analyses were performed on the samples to identify their compositional characteristics. [Pg.274]

In associating the r-process with supernova explosions, several attempts to go beyond the canonical and MER models have been made by taking into account some evolution of the characteristics of the sites of the r-process during its development. These models are coined dynamical (DYR) in the following in order to remind of the time variations of the thermodynamic state of the r-process environment (see [24] for references). These models do not rely on any specific explosion scenario. They just assume that a material that is initially hot enough for allowing a nuclear statistical equilibrium (NSE) to be achieved expands and cools in a prescribed way on some selected timescale. This evolution is fully parameterized. [Pg.314]

The essential nature of this relationship is clear statistical theories are based on a number of simplifying assumptions consistent with chaotic behavior. Specifically,2 any such theory must satisfy microscopic reversibility and the condition of zero relevance. The latter condition requires that the final state be independent of all initial conditions other than conserved quantities, that is, from the viewpoint of classical mechanics, that the system display the relaxation characteristic of chaotic motion. We note, for reference, that this minimal set of requirements allows for the construction of a large number of theories,3 the most prominant of which are the RRK.M theory of uni-molecular dissociation4 and the phase space theory of bimolecular reactions.5 Such theories have analogues, and in some cases their origins are in other areas such as nuclear physics.6... [Pg.366]

Electron spin echo spectroscopy (ESE) monitors the spontaneous generation of microwave energy as a function of the timing of a specific excitation scheme, i.e. two or more short resonant microwave pulses. This is illustrated in Fig. 7. In a typical two-pulse excitation, the initial n/2 pulse places the spin system in a coherent state. Subsequently, the spin packets, each characterized by their own Larmor precession frequency m, start to dephase. A second rx-pulse at time r effectively reverses the time evolution of the spin packet magnetizations, i.e. the spin packets start to rephase, and an emission of microwave energy (the primary echo) occurs at time 2r. The echo ampHtude, as a fvmction of r, constitutes the ESE spectrum and relaxation processes lead to an irreversible loss of phase correlation. The characteristic time for the ampHtude decay is called the phase memory time T. This decay is often accompanied by a modulation of the echo amplitude, which is due to weak electron-nuclear hyperfine interactions. The analysis of the modulation frequencies and ampHtudes forms the basis of the electron spin echo envelope modulation spectroscopy (ESEEM). [Pg.310]

The production of radionuclides in meteoroids that are orbiting the Sun takes place by nuclear spallation and neutron-capture reactions with the atoms of the major elements (Bogard et al. 1995 Leya et al. 2000). The concentration of a particular radionuclide in a stony meteoroid exposed to cosmic rays in Fig. 18.14 initially increases with time until it reaches a state of equilibrium or saturation when its rate of decay is equal to its rate of production. When such a meteoroid enters the atmosphere of the Earth and explodes, the resulting meteorite specimens are assumed to be saturated with respect to the cosmogenic radionuclides they contain. After a meteorite has landed on the surface of the Earth, the production of radionuclides stops because the Earth is protected from cosmic rays by its magnetic field and by the atmosphere. Therefore, the rate of decay of cosmogenic radionuclides decreases with time as each nuclide continues to decay with its characteristic halflife. The terrestrial age of a meteorite specimen collected in Antarctica or anywhere else on the Earth is calculated from the rates of decay of the radionuclides (e.g., C1 or A1) that remain at the time of analysis (Jull 2001). [Pg.655]

The resonantly scattered radiation may interfere with the radiation scattered by electrons of the atom. The characteristic time - the lifetime of nuclear excited state T oc r i - is longer by several orders of magnitude than the lattice vibration periods. There is no correlation here between the initial and final positions of the atom. Despite this, the scattered wave remains coherent with the incident one. [Pg.180]


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