Radioactive fallout particles, formation

Touring the formation of radioactive fallout particles, one of the most important processes is the uptake, in the cooling nuclear fireball, of the vaporized radioactive fission products by particles of molten soil or other environmental materials. Owing to the differences in the chemical nature of the various radioactive elements, their rates of uptake vary, depending upon temperature, pressure, and substrate and vapor-phase composition. These varying rates of uptake, combined with different residence times of the substrate particles in the fireball, result in radiochemical fractionation of the fallout. This fractionation has a considerable effect on the final partition of radioactivity, exposure rate, and radionuclides between the ground surface and the atmosphere. 

Table II summarizes some of the features of the radioactive fallout processes in geophysical and astronomical settings. It seems that similarities do exist between the processes of formation of single particles from nuclear explosions and formation of the solar system from the debris of supernova explosion. We may be able to learn much more about the origin of the earth, by further investigating the process of radioactive fallout from the nuclear weapons tests.

This paper deals mainly with the condensation of trace concentrations of radioactive vapor onto spherical particles of a substrate. For this situation the relation between the engineering approach, the molecular approach, and the fluid-dynamic approach are illustrated for several different cases of rate limitation. From these considerations criteria are derived for the use of basic physical and chemical parameters to predict the rate-controlling step or steps. Finally, the effect of changing temperature is considered and the groundwork is thereby laid for a kinetic approach to predicting fallout formation. The relation of these approaches to the escape of fission products from reactor fuel and to the deposition of radon and thoron daughters on dust particles in a uranium mine is indicated. 

FALLOUT (Radioactive . The term fallout generally has been used to refer to particulate mutter that is thrown into the atmosphere by a nuclear process of short time duration. Primary examples are nuclear weapon debris and effluents from a nuclear reactor excursion. The name fallout is applied both to matter that is aloll and to matter that has been deposited on the surface of the earfh. Depending on the conditions of formation, this material ranges in texture from an aerosol to granules uf considerable size. The aerodynamic principles governing tls deposition are the same as for any Other material of comparable physical nature that is thrown into the air. such as volcanic ash or particles from chimneys. Therefore, many of the principles learned in. studies of fallout from nuclear weapons can be applied lo studies of other particulate pollution in the atmosphere. 

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