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This equation has been used by Sundstrom and coworkers [151] and adapted to the analysis of femtosecond spectral evolution as monitored by the bond-twisting events in barrierless isomerization in solution. The theoretical derivation of Aberg et al. establishes a link between the Smoluchowski equation with a sink and the Schrodinger equation of a solute coupled to a thermal bath. The reader is referred to this important work for further theoretical details and a thorough description of the experimental set up. It is sufficient to say here that the classical link is established via the Hamilton-Jacobi equation formalism. By using the standard ansatz Xn(X,t)= A(X,i)cxp(S(X,t)/i1l), where S(X,t) is the action of the dynamical system, and neglecting terms in once this... [Pg.312]

Hence, the suggested approaches do not allow solving the problem of the internal links distribution for a polymer chain completely. In the present work we propose its analytic solution in terms of SARWstrict statistics, that is, without taking into account of the so-called volume interaction. [Pg.4]

Pasteur s work was linked to that of his older friend and colleague, the physicist Jean Baptiste Biot (1774—1862). He was a pioneer of polarimetry and showed that certain solid quartz crystals, and later solutions of sugars, rotated the plane of polarized light in opposite directions. He realized this must be a molecular property and suggested the term optical activity for the phenomenon. The work of these two scientists complemented each other and the phenomenon has immense significance, particularly in a biological context. [Pg.708]


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