Three-dimensional femtosecond time-resolved

The question is then, first, how often has such a complete match between experiment and theoretical simulation been achieved Second, are there good examples where complete simulations have been carried out but lead to two or more equally acceptable models to interpret the experimental results I refer to this question of ambiguity also in relation to a very similar problem arising in the interpretation of nontime-resolved high-resolution spectroscopy data [1,2], which provided in fact, the first experimental results on nontrivial three-dimensional wavepacket motion on the femtosecond time scale [3]. 

Beyond imaging, the combination of CRS microscopy with spectroscopic techniques has been used to obtain the full wealth of the chemical and the physical structure information of submicron-sized samples. In the frequency domain, multiplex CRS microspectroscopy allows the chemical identification of molecules on the basis of their characteristic Raman spectra and the extraction of their physical properties, e.g., their thermodynamic state. In the time domain, time-resolved CRS microscopy allows the recording of the localized Raman free induction decay occurring on the femtosecond and picosecond time scales. CRS correlation spectroscopy can probe three-dimensional diffusion dynamics with chemical selectivity. 

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