Electron and nucleus dynamics tracked with pulse train in time-resolved photoelectron spectroscopy

6 Electron and nucleus dynamics tracked with pulse train in time-resolved photoelectron spectroscopy [Pg.167]

In this section we try to practically realize the idea of Ref. [20] by applying a train of subfemtosecond pulses composed of frequencies appropriate to photoelectron spectroscopy. Just as the vibrational progression is clearly recorded in conventional (time-independent) photoelectron spectra, time-resolved photoelectron spectroscopy with a well designed pulse train is anticipated to be able to monitor the electronic state progression along with signatures of the nuclear vibrational d mamics. [Pg.168]