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Indirect photodissociation Resonances and recurrences

The main characteristics of indirect dissociation are resonances in the time-independent picture and recurrences in the time-dependent approach. Resonances and recurrences are the two sides of one coin they reveal the same dynamical information but provide different explanations and points of view. To begin this chapter we discuss in Section 7.1, on a qualitative level, indirect photodissociation of a one-dimensional system. A more quantitative analysis follows in Section 7.2. The time-dependent and the time-independent views of indirect photodissociation are outlined and illustrated in Sections 7.3 and 7.4, respectively, with emphasis on vibrational excitation of the NO moiety in the photodissociation of CH30N0(S i). Section 7.5 accentuates the relation between [Pg.134]

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Photodissociations

Recurrence

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