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Singlet-triplet branching ratio

Wade, E.A., H. Clauberg, S. K. Kim, A. Mellinger, and C.B. Moore (1997a), Dynamics of rotational energy release for dissociation of singlet ketene and the singlet/triplet branching ratio, J. Phys. Chem. A, 101, 732-739. [Pg.1470]

The ZEKE-PFI spectrum, recorded from the HC1 F1 A intermediate state, shows a completely different 2II1/2/2II3/2 subband branching ratio, equal to 0.12 (de Beer, et al., 1990 and Fig. 8.21, upper panel). A calculation, using the BOS formalism (see Section 8.1.1) with ab initio transition moments and a singlet-triplet mixing of 22% reproduces the ratio observed by conventional spectroscopy but not that in the ZEKE spectrum (Fig. 8.21, middle panel). [Pg.593]

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See also in sourсe #XX -- [ Pg.519 ]



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Singlet-triplet

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