Polarisation vector nature

When the vector properties of the scattered fragments are correlated, both the integrated intensities and the resolved Doppler profiles are profoundly sensitive to changes in the relative directors and polarisations of the photolysis (1, p) and probe/analysis (ka, j ) laser beams and to the nature of the probed transition, P, Rt or Qt. Alternative quantal and classical procedures for relating the observed changes to the vector correlations have been developed by Dixon [6] and by Houston and his co-workers [47,49] and these have already been used to andyse the photodissociation dynamics in H2O2 [21,22,23], SCO [48,50], (HCO)2 HNO3 [23], NNO... 

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