Photon capture, direct molecular dynamics

Photon capture, direct molecular dynamics, adiabatic systems, initial conditions, 373-377... 

The discussion above must be modified if the acceptor molecules adsorb onto the electrode surface. Under these circumstances, the electrons are captured by the acceptor directly rather than through an intermediary solvated electron, and such direct photoassisted electron transfer has been much studied recently with the advent of dye-sensitized solar cells and molecular electronic devices. The normal approach is to use two-photon excitation both to probe the existence of localized states at the surface and to explore their dynamics. In experiments of this nature, which have been mostly carried out on ad-... 

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