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Doorway wavepacket fluorescence

The first term in Eq. (4.3) is reminiscent of Eq. (3.2) for the spontaneous emission spectrum. It represents a doorway wavepacket created by the pump in the excited state, which is then detected by its overlap with a window. The only difference is that the role of the gate in determining the window in SLE is now played by the probe Wigner function W2. In addition, the pump-probe signal contains a second term that does not show up in fluorescence. This term represents a wavepacket created in the ground state (a hole ) that evolves in time as well and is finally determined by a different window Wg [24]. In the snapshot limit, defined in the preceding section, we have... [Pg.357]

Appendix C Four-Point Correlation Function Expression for Fluorescence Spectra Appendix D Phase-Space Doorway-Window Wavepackets for Fluorescence Appendix E Doorway-Window Phase-Space Wavepackets for Pump-Probe Signals References... [Pg.345]

APPENDIX D PHASE-SPACE DOORWAY-WINDOW WAVEPACKETS FOR FLUORESCENCE... [Pg.367]

We now derive the expression for the fluorescence signal in terms of the doorway and window wavepackets instead of the four-point correlation function. We start with Eq. (3.1) and write the four-point correlation function F(4) explicitly as the trace with respect to the equilibrium density matrix. We then use the cyclic invariance of the trace and obtain... [Pg.367]


See also in sourсe #XX -- [ Pg.368 ]




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